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- Experimental investigation of excitonic spin relaxation dynamics in GaN doi link

Auteur(s): Brimont C., Gallart Mathieu, Cregut Olivier, Honerlage Bernd, Gilliot Pierre

(Article) Publié: Physical Review B, vol. 77 p.125201 (2008)


Ref HAL: hal-00545182_v1
DOI: 10.1103/PhysRevB.77.125201
WoS: 000254543000054
Exporter : BibTex | endNote
21 Citations
Résumé:

By performing nondegenerate pump- probe experiments, we study the relaxation dynamics of spin- polarized A and B excitons in wurtzite epitaxial GaN. By analyzing the differential reflectivity spectra (Delta R/R) of the two circularly polarized probe components, we are able to identify each spin relaxation channel ( electron, light- and heavy- hole spin flips ) separately and to extract characteristic times of the different spin relaxation processes. In addition, spectral oscillatory features are observed for negative delays. They show a rapid rise determined by the fast dephasing time T-2 of the excitonic transitions. We show that the high density of dislocations increases the spin relaxation of electrons and holes through the Elliot - Yafet mechanism and makes the exciton dephasing time very short. The measured heavy- hole relaxation time, which is not extremely short compared to the electron relaxation time, can be related to the band structure, in which the degeneracy between different spin valence bands is partially lifted.