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Understanding and controlling the dynamical, electronic and magnetic properties of carbon-based materials is of fundamental relevance for employing these structures in future nano- and bioscience applications. In this talk, we report on the recent discoveries obtained in these new hybrid materials with a special focus on results obtained by solid state nuclear magnetic resonance spectroscopy. These studies provide a new insight into such structures and allow to model some of their exotic properties. Our contribution to the knowledge of 1D-confined molecules address more general topics on the confinement that profoundly changes the properties of matter and the opportunity to engineer nano-systems. Some potential applications of these new hybrid materials in nuclear magnetic resonance spectroscopy and imaging will be presented.