--------------------
- Connecting packing efficiency of binary hard sphere systems to their intermediate range structure doi link

Auteur(s): Yuan H., Zhang Z., Kob W.(Corresp.), Wang Y.

(Article) Publié: Physical Review Letters, vol. 127 p.278001 (2022)
Texte intégral en Openaccess : arxiv


Ref HAL: hal-03522429_v1
DOI: 10.1103/PhysRevLett.127.278001
Exporter : BibTex | endNote
Résumé:

Using computed x-ray tomography we determine the three dimensional (3D) structure of binary hard sphere mixtures as a function of composition and size ratio of the particles q. Using a recently introduced four-point correlation function we reveal that this 3D structure has on intermediate and large length scales a surprisingly regular order, the symmetry of which depends on q. The related structural correlation length has a minimum at the composition at which the packing fraction is highest. At this composition also the number of different local particle arrangements has a maximum, indicating that efficient packing of particles is associated with a structure that is locally maximally disordered.