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- Detection of second-order nonlinear optical magnetization by mapping normalized Stokes parameters doi link

Auteur(s): Bovino Fabio Antonio, Larciprete Maria Cristina, Sibilia Concita, Leahu Gregory, Váro György, Gergely C.

(Article) Publié: Journal Of The Optical Society Of America B, vol. 30 p.568 (2013)
Texte intégral en Openaccess : openaccess


Ref HAL: hal-00788841_v1
DOI: 10.1364/JOSAB.30.000568
WoS: 000315603400013
Exporter : BibTex | endNote
5 Citations
Résumé:

A measurable magnetic (nonlocal) contribution to the second harmonic generation (SHG) of nonmagnetic materi- als is an intriguing issue related to chiral materials, such as biomolecules. Here we report the detection of an intensity-dependent optically induced magnetization of a chiral bacteriorhodopsin film under femtosecond pulse excitation (830 nm) and far from the material's resonance. The analysis of the pump intensity-dependent noncol- linear SHG signal, by means of the polarization map of normalized Stokes parameters, allows one to improve the detection of the nonlinear optical magnetization M 2ω contribution to the SHG signal.