
Domaines de Recherche: - Physique/Matière Condensée/Mécanique statistique
- Physique/Matière Condensée/Matière Molle
- Physique/Matière Condensée/Systèmes désordonnés et réseaux de neurones
- Physique/Matière Condensée/Science des matériaux
- Physique/Physique/Chimie-Physique
- Physique/Matière Condensée
- Physique/Physique/Physique Générale
- Physique/Physique/Biophysique
- Physique/Physique/Physique Numérique
- Physique
- Physique/Mécanique/Mécanique des matériaux
- Physique/Mécanique/Mécanique des solides
- Physique/Matière Condensée/Electrons fortement corrélés
- Physique/Matière Condensée/Autre
- Mathématiques/Probabilités [math.PR]
- Mathématiques/Statistiques [math.ST]
- Statistiques/Théorie [stat.TH]
- Sciences de l'ingénieur/Mécanique/Vibrations
- Physique/Mécanique/Vibrations
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La dynamique lente des matériaux vitreux
Auteur(s): Berthier L.
(H.D.R.)
, 2008 | |
Dernieres productions scientifiques :

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Microscopic observation of two-level systems in a metallic glass model 
Auteur(s): Mocanu Felix, Berthier L., Ciarella Simone, Khomenko Dmytro, Reichman David, Scalliet C., Zamponi Francesco
(Article) Publié:
The Journal Of Chemical Physics, vol. 158 p.014501 (2023)
Texte intégral en Openaccess : 
Ref HAL: hal-03920514_v1
Ref Arxiv: 2209.09579
DOI: 10.1063/5.0128820
Ref. & Cit.: NASA ADS
Exporter : BibTex | endNote
Résumé: The low-temperature quasi-universal behavior of amorphous solids has been attributed to the existence of spatially localized tunneling defects found in the low-energy regions of the potential energy landscape. Computational models of glasses can be studied to elucidate the microscopic nature of these defects. Recent simulation work has demonstrated the means of generating stable glassy configurations for models that mimic metallic glasses using the swap Monte Carlo algorithm. Building on these studies, we present an extensive exploration of the glassy metabasins of the potential energy landscape of a variant of the most widely used model of metallic glasses. We carefully identify tunneling defects and reveal their depletion with increased glass stability. The density of tunneling defects near the experimental glass transition temperature appears to be in good agreement with experimental measurements.
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Thirty milliseconds in the life of a supercooled liquid 
Auteur(s): Scalliet C., Guiselin B., Berthier L.
(Article) Publié:
Physical Review X, vol. p.041028 (2022)
Texte intégral en Openaccess : 
Ref HAL: hal-03915196_v1
Ref Arxiv: 2207.00491
DOI: 10.1103/PhysRevX.12.041028
Ref. & Cit.: NASA ADS
Exporter : BibTex | endNote
Résumé: We combine the swap Monte Carlo algorithm to long multi-CPU molecular dynamics simulations to analyse the equilibrium relaxation dynamics of model supercooled liquids over a time window covering ten orders of magnitude for temperatures down to the experimental glass transition temperature $T_g$. The analysis of \rev{several} time correlation functions coupled to spatio-temporal resolution of particle motion allow us to elucidate the nature of the equilibrium dynamics in deeply supercooled liquids. We find that structural relaxation starts at early times in rare localised regions characterised by a waiting time distribution that develops a power law near $T_g$. At longer times, relaxation events accumulate with increasing probability in these regions as $T_g$ is approached. This accumulation leads to a power-law growth of the linear extension of relaxed domains with time with a large, temperature-dependent dynamic exponent. Past the average relaxation time, unrelaxed domains slowly shrink with time due to relaxation events happening at their boundaries. Our results provide a complete microscopic description of the particle motion responsible for key experimental signatures of glassy dynamics, from the shape and temperature evolution of relaxation spectra to the core features of dynamic heterogeneity. They also provide a microscopic basis to understand the emergence of dynamic facilitation in deeply supercooled liquids and allow us to critically reassess theoretical descriptions of the glass transition.
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Is glass a state of matter? 
Auteur(s): Guiselin B., Tarjus Gilles, Berthier L.
(Article) Publié:
Physics And Chemistry Of Glasses: European Journal Of Glass Science And Technology Part B, vol. p.136 (2022)
Texte intégral en Openaccess : 
Ref HAL: hal-03915194_v1
Ref Arxiv: 2207.14204
DOI: 10.13036/17533562.63.5.15
Ref. & Cit.: NASA ADS
Exporter : BibTex | endNote
Résumé: Glass is everywhere. We use and are surrounded by glass objects which make tangible the reality of glass as a distinct state of matter. Yet, glass as we know it is usually obtained by cooling a liquid sufficiently rapidly below its melting point to avoid crystallisation. The viscosity of this supercooled liquid increases by many orders of magnitude upon cooling, until the liquid becomes essentially arrested on experimental timescales below the ``glass transition'' temperature. From a structural viewpoint, the obtained glass still very much resembles the disordered liquid, but from a mechanical viewpoint, it is as rigid as an ordered crystal. Does glass qualify as a separate state of matter? We provide a pedagogical perspective on this question using basic statistical mechanical concepts. We recall the definitions of states of matter and of phase transitions between them. We review recent theoretical results suggesting why and how an ``ideal glass'' can indeed be defined as a separate equilibrium state of matter. We discuss recent success of computer simulations trying to analyse this glass state. We close with some experimental perspectives.
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Collective dynamics in a glass-former with Mari-Kurchan interactions 
Auteur(s): Nishikawa Y., Ikeda A., Berthier L.
(Article) Publié:
The Journal Of Chemical Physics, vol. p.244503 (2022)
Texte intégral en Openaccess : 
Ref HAL: hal-03807702_v1
Ref Arxiv: 2204.05130
DOI: 10.1063/5.0096356
Ref. & Cit.: NASA ADS
Exporter : BibTex | endNote
Résumé: We numerically study the equilibrium relaxation dynamics of a two-dimensional Mari-Kurchan glass model. The tree-like structure of particle interactions forbids both non-trivial structural motifs and the emergence of a complex free-energy landscape leading to a thermodynamic glass transition, while the finite-dimensional nature of the model prevents the existence of a mode-coupling singularity. Nevertheless, the equilibrium relaxation dynamics is shown to be in excellent agreement with simulations performed in conventional glass-formers. Averaged time-correlation functions display a phenomenology typical of supercooled liquids, including the emergence of an excess signal in relaxation spectra at intermediate frequencies. We show that this evolution is accompanied by strong signatures of collective and heterogeneous dynamics which cannot be interpreted in terms of single particle hopping and emerge from dynamic facilitation. Our study demonstrates that an off-lattice interacting particle model with extremely simple structural correlations displays quantitatively realistic glassy dynamics.
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Disordered collective motion in dense assemblies of persistent particles 
Auteur(s): Keta Y.-E., Jack Robert L., Berthier L.
(Article) Publié:
Physical Review Letters, vol. p.048002 (2022)
Texte intégral en Openaccess : 
Ref HAL: hal-03775859_v1
Ref Arxiv: 2201.04902
DOI: 10.1103/PhysRevLett.129.048002
Ref. & Cit.: NASA ADS
Exporter : BibTex | endNote
Résumé: We explore the emergence of nonequilibrium collective motion in disordered non-thermal active matter when persistent motion and crowding effects compete, using simulations of a two-dimensional model of size polydisperse self-propelled particles. In stark contrast with monodisperse systems, we find that polydispersity stabilizes a homogeneous active liquid at arbitrary large persistence times, characterized by remarkable velocity correlations and irregular turbulent flows. For all persistence values, the active fluid undergoes a nonequilibrium glass transition at large density. This is accompanied by collective motion, whose nature evolves from near-equilibrium spatially heterogeneous dynamics at small persistence, to a qualitatively different intermittent dynamics when persistence is large. This latter regime involves a complex time evolution of the correlated displacement field
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